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Carbon nanotube photo- and electroluminescence in longitudinal electric fields

  • Marcus Freitag
  • , Mathias Steiner
  • , Anton Naumov
  • , Joshua P. Small
  • , Ageeth A. Bol
  • , Vasili Perebeinos
  • , Phaedon Avouris

Research output: Contribution to journalArticlepeer-review

43 Scopus citations

Abstract

The photoluminescence of a partially suspended, semiconducting carbon nanotube that forms the active channel of a field-effect transistor is quenched and red-shifted upon application of a longitudinal electrical (source-drain) field. The quenching can be explained by a loss of oscillator strength and an increased Auger-like nonradiative decay of the E11 exciton. The spectral shifts are due to drain-field-induced doping that leads to enhanced dielectric screening. Electroluminescence due to electron impact excitation of E11 excitons is red-shifted and broadened with respect to the zero-field photoluminescence. A combination of screening and heating of the carbon nanotube can explain both spectral shift and broadening of the electrically induced light emission.

Original languageEnglish
Pages (from-to)3744-3748
Number of pages5
JournalACS Nano
Volume3
Issue number11
DOIs
StatePublished - Nov 24 2009

Keywords

  • Carbon nanotube
  • Doping
  • Electroluminescence
  • Excitons
  • Field-effect transistor
  • Nanophotonics
  • Optoelectronics
  • Photoluminescence
  • Screening

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