Skip to main navigation Skip to search Skip to main content

Epitaxial phase transformation between cylindrical and double gyroid mesophases

  • Lei Zhu
  • , Lu Sun
  • , Jianjun Miao
  • , Li Cui
  • , Qing Ge
  • , Roderic P. Quirk
  • , Chenchen Xue
  • , Stephen Z.D. Cheng
  • , Benjamin S. Hsiao
  • , Carlos A. Avila-Orta
  • , Igors Sics
  • , Marie E. Cantino

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

Abstract

Complex phase transformation between the hexagonal cylinder (Hex) and double gyroid (G) phases in a polystyrene-block-poly(ethylene oxide) (PS-b-PEO) diblock copolymer was investigated using two-dimensional (2D) synchrotron small-angle X-ray scattering (SAXS), and transmission electron microscope (TEM). The PS-b-PEO sample contained a small population of another bicontinuous cubic phase having an Im3̄m symmetry. These two bicontinuous cubic phases (G and Im3̄m) had the same unit cell dimensions. Under a large-amplitude reciprocating shear, the bicontinuous cubic phases transformed into a "single-crystal"-like Hex phase. When annealed at 150°C for 40 min, the Hex phase partially transformed into well-oriented twinned structures of the G and Im3̄m phases without significant loss of orientation in 2D SAXS measurements. Epitaxial phase transformation relationships between the Hex/G and Hex/ Im3̄m phases were identified. The mechanism of the Hex → G transformation was examined by TEM.

Original languageEnglish
Title of host publicationMulticomponent Polymer Systems
Subtitle of host publicationPhase Behavior, Dynamics and Applications
PublisherMaterials Research Society
Pages8-13
Number of pages6
ISBN (Print)155899808X, 9781558998087
DOIs
StatePublished - 2004
Event2004 MRS Fall Meeting - Boston. MA, United States
Duration: Nov 29 2004Dec 3 2004

Publication series

NameMaterials Research Society Symposium Proceedings
Volume856

Conference

Conference2004 MRS Fall Meeting
Country/TerritoryUnited States
CityBoston. MA
Period11/29/0412/3/04

Fingerprint

Dive into the research topics of 'Epitaxial phase transformation between cylindrical and double gyroid mesophases'. Together they form a unique fingerprint.

Cite this