Graphene and Beyond: Recent Advances in Two-Dimensional Materials Synthesis, Properties, and Devices

Yu Lei; Tianyi Zhang; Yu Chuan Lin; Tomotaroh Granzier-Nakajima; George Bepete; Dorota A. Kowalczyk; Zhong Lin; Da Zhou; Thomas F. Schranghamer; Akhil Dodda; Amritanand Sebastian; Yifeng Chen; Yuanyue Liu; Geoffrey Pourtois; Thomas J. Kempa; Bruno Schuler; Mark T. Edmonds; Su Ying Quek; Ursula Wurstbauer; Stephen M. Wu; Nicholas R. Glavin; Saptarshi Das; Saroj Prasad Dash; Joan M. Redwing; Joshua A. Robinson; Mauricio Terrones

doi:10.1021/acsnanoscienceau.2c00017

Graphene and Beyond: Recent Advances in Two-Dimensional Materials Synthesis, Properties, and Devices

Yu Lei
, Tianyi Zhang
, Yu Chuan Lin
, Tomotaroh Granzier-Nakajima
, George Bepete
, Dorota A. Kowalczyk
, Zhong Lin
, Da Zhou
, Thomas F. Schranghamer
, Akhil Dodda
, Amritanand Sebastian
, Yifeng Chen
, Yuanyue Liu
, Geoffrey Pourtois
, Thomas J. Kempa
, Bruno Schuler
, Mark T. Edmonds
, Su Ying Quek
, Ursula Wurstbauer
, Stephen M. Wu

Nicholas R. Glavin, Saptarshi Das, Saroj Prasad Dash, Joan M. Redwing, Joshua A. Robinson, Mauricio Terrones

Physics

Binghamton University

Pennsylvania State University
Tsinghua University
University of Lodz
National University of Singapore
University of Texas at Austin
Interuniversitair Micro-Elektronica Centrum
Johns Hopkins University
Swiss Federal Laboratories for Materials Science and Technology (Empa)
Monash University
University of Münster
University of Rochester
Air Force Research Laboratory
Chalmers University of Technology
Shinshu University

Research output: Contribution to journal › Review article › peer-review

204 Scopus citations

Abstract

Since the isolation of graphene in 2004, two-dimensional (2D) materials research has rapidly evolved into an entire subdiscipline in the physical sciences with a wide range of emergent applications. The unique 2D structure offers an open canvas to tailor and functionalize 2D materials through layer number, defects, morphology, moiré pattern, strain, and other control knobs. Through this review, we aim to highlight the most recent discoveries in the following topics: theory-guided synthesis for enhanced control of 2D morphologies, quality, yield, as well as insights toward novel 2D materials; defect engineering to control and understand the role of various defects, including in situ and ex situ methods; and properties and applications that are related to moiré engineering, strain engineering, and artificial intelligence. Finally, we also provide our perspective on the challenges and opportunities in this fascinating field.

Original language	English
Pages (from-to)	450-485
Number of pages	36
Journal	ACS Nanoscience Au
Volume	2
Issue number	6
DOIs	https://doi.org/10.1021/acsnanoscienceau.2c00017
State	Published - Dec 21 2022

Keywords

2D Materials
Artificial Intelligence
Defect Engineering
Excitonic Properties
Magnetic and Topological Properties
Moiré Engineering
Strain Engineering
Theory-Guided Synthesis

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10.1021/acsnanoscienceau.2c00017

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Lei, Y., Zhang, T., Lin, Y. C., Granzier-Nakajima, T., Bepete, G., Kowalczyk, D. A., Lin, Z., Zhou, D., Schranghamer, T. F., Dodda, A., Sebastian, A., Chen, Y., Liu, Y., Pourtois, G., Kempa, T. J., Schuler, B., Edmonds, M. T., Quek, S. Y., Wurstbauer, U., ... Terrones, M. (2022). Graphene and Beyond: Recent Advances in Two-Dimensional Materials Synthesis, Properties, and Devices. ACS Nanoscience Au, 2(6), 450-485. https://doi.org/10.1021/acsnanoscienceau.2c00017

@article{da25c43cf6634940a3378ad19cbcf88a,

title = "Graphene and Beyond: Recent Advances in Two-Dimensional Materials Synthesis, Properties, and Devices",

abstract = "Since the isolation of graphene in 2004, two-dimensional (2D) materials research has rapidly evolved into an entire subdiscipline in the physical sciences with a wide range of emergent applications. The unique 2D structure offers an open canvas to tailor and functionalize 2D materials through layer number, defects, morphology, moir{\'e} pattern, strain, and other control knobs. Through this review, we aim to highlight the most recent discoveries in the following topics: theory-guided synthesis for enhanced control of 2D morphologies, quality, yield, as well as insights toward novel 2D materials; defect engineering to control and understand the role of various defects, including in situ and ex situ methods; and properties and applications that are related to moir{\'e} engineering, strain engineering, and artificial intelligence. Finally, we also provide our perspective on the challenges and opportunities in this fascinating field.",

keywords = "2D Materials, Artificial Intelligence, Defect Engineering, Excitonic Properties, Magnetic and Topological Properties, Moir{\'e} Engineering, Strain Engineering, Theory-Guided Synthesis",

author = "Yu Lei and Tianyi Zhang and Lin, \{Yu Chuan\} and Tomotaroh Granzier-Nakajima and George Bepete and Kowalczyk, \{Dorota A.\} and Zhong Lin and Da Zhou and Schranghamer, \{Thomas F.\} and Akhil Dodda and Amritanand Sebastian and Yifeng Chen and Yuanyue Liu and Geoffrey Pourtois and Kempa, \{Thomas J.\} and Bruno Schuler and Edmonds, \{Mark T.\} and Quek, \{Su Ying\} and Ursula Wurstbauer and Wu, \{Stephen M.\} and Glavin, \{Nicholas R.\} and Saptarshi Das and Dash, \{Saroj Prasad\} and Redwing, \{Joan M.\} and Robinson, \{Joshua A.\} and Mauricio Terrones",

note = "Publisher Copyright: {\textcopyright} 2022 American Chemical Society.",

year = "2022",

month = dec,

day = "21",

doi = "10.1021/acsnanoscienceau.2c00017",

language = "English",

volume = "2",

pages = "450--485",

journal = "ACS Nanoscience Au",

issn = "2694-2496",

publisher = "American Chemical Society",

number = "6",

}

Lei, Y, Zhang, T, Lin, YC, Granzier-Nakajima, T, Bepete, G, Kowalczyk, DA, Lin, Z, Zhou, D, Schranghamer, TF, Dodda, A, Sebastian, A, Chen, Y, Liu, Y, Pourtois, G, Kempa, TJ, Schuler, B, Edmonds, MT, Quek, SY, Wurstbauer, U, Wu, SM, Glavin, NR, Das, S, Dash, SP, Redwing, JM, Robinson, JA & Terrones, M 2022, 'Graphene and Beyond: Recent Advances in Two-Dimensional Materials Synthesis, Properties, and Devices', ACS Nanoscience Au, vol. 2, no. 6, pp. 450-485. https://doi.org/10.1021/acsnanoscienceau.2c00017

TY - JOUR

T1 - Graphene and Beyond

T2 - Recent Advances in Two-Dimensional Materials Synthesis, Properties, and Devices

AU - Lei, Yu

AU - Zhang, Tianyi

AU - Lin, Yu Chuan

AU - Granzier-Nakajima, Tomotaroh

AU - Bepete, George

AU - Kowalczyk, Dorota A.

AU - Lin, Zhong

AU - Zhou, Da

AU - Schranghamer, Thomas F.

AU - Dodda, Akhil

AU - Sebastian, Amritanand

AU - Chen, Yifeng

AU - Liu, Yuanyue

AU - Pourtois, Geoffrey

AU - Kempa, Thomas J.

AU - Schuler, Bruno

AU - Edmonds, Mark T.

AU - Quek, Su Ying

AU - Wurstbauer, Ursula

AU - Wu, Stephen M.

AU - Glavin, Nicholas R.

AU - Das, Saptarshi

AU - Dash, Saroj Prasad

AU - Redwing, Joan M.

AU - Robinson, Joshua A.

AU - Terrones, Mauricio

PY - 2022/12/21

Y1 - 2022/12/21

N2 - Since the isolation of graphene in 2004, two-dimensional (2D) materials research has rapidly evolved into an entire subdiscipline in the physical sciences with a wide range of emergent applications. The unique 2D structure offers an open canvas to tailor and functionalize 2D materials through layer number, defects, morphology, moiré pattern, strain, and other control knobs. Through this review, we aim to highlight the most recent discoveries in the following topics: theory-guided synthesis for enhanced control of 2D morphologies, quality, yield, as well as insights toward novel 2D materials; defect engineering to control and understand the role of various defects, including in situ and ex situ methods; and properties and applications that are related to moiré engineering, strain engineering, and artificial intelligence. Finally, we also provide our perspective on the challenges and opportunities in this fascinating field.

AB - Since the isolation of graphene in 2004, two-dimensional (2D) materials research has rapidly evolved into an entire subdiscipline in the physical sciences with a wide range of emergent applications. The unique 2D structure offers an open canvas to tailor and functionalize 2D materials through layer number, defects, morphology, moiré pattern, strain, and other control knobs. Through this review, we aim to highlight the most recent discoveries in the following topics: theory-guided synthesis for enhanced control of 2D morphologies, quality, yield, as well as insights toward novel 2D materials; defect engineering to control and understand the role of various defects, including in situ and ex situ methods; and properties and applications that are related to moiré engineering, strain engineering, and artificial intelligence. Finally, we also provide our perspective on the challenges and opportunities in this fascinating field.

KW - 2D Materials

KW - Artificial Intelligence

KW - Defect Engineering

KW - Excitonic Properties

KW - Magnetic and Topological Properties

KW - Moiré Engineering

KW - Strain Engineering

KW - Theory-Guided Synthesis

UR - https://www.scopus.com/pages/publications/85139295630

U2 - 10.1021/acsnanoscienceau.2c00017

DO - 10.1021/acsnanoscienceau.2c00017

M3 - Review article

SN - 2694-2496

VL - 2

SP - 450

EP - 485

JO - ACS Nanoscience Au

JF - ACS Nanoscience Au

IS - 6

ER -

Graphene and Beyond: Recent Advances in Two-Dimensional Materials Synthesis, Properties, and Devices

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Keywords

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