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Phase modulation of ultrashort light pulses using molecular rotational wave packets

  • R. A. Bartels
  • , T. C. Weinacht
  • , N. Wagner
  • , M. Baertschy
  • , Chris H. Greene
  • , M. M. Murnane
  • , H. C. Kapteyn

Research output: Contribution to journalArticlepeer-review

264 Scopus citations

Abstract

The time-dependent phase modulation of ultrashort light pulses using molecular rotational wave packets was studied. The bandwidth of a probe pulse was increased by a factor of 9, by using impulsively excited rotational wave packets in CO2. The negative chirp induced was removed by propagation through a fused silica window, without the use of a pulse compressor. The technique is applied for optical phase modulation over a broad spectral region varying from the infrared to the ultraviolet range.

Original languageEnglish
Pages (from-to)139031-139034
Number of pages4
JournalPhysical Review Letters
Volume88
Issue number1
StatePublished - Jan 7 2002

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