Role of water in electron-initiated processes and radical chemistry: Issues and scientific advances

Bruce C. Garrett; David A. Dixon; Donald M. Camaioni; Daniel M. Chipman; Mark A. Johnson; Charles D. Jonah; Gregory A. Kimmel; John H. Miller; Thomas N. Rescigno; Peter J. Rossky; Sotiris S. Xantheas; Steven D. Colson; Allan H. Laufer; Douglas Ray; Paul F. Barbara; David M. Bartels; Kurt H. Becker; Kit H. Bowen; Stephen E. Bradforth; Ian Carmichael; James V. Coe; L. Rene Corrales; James P. Cowin; Michel Dupuis; Kenneth B. Eisenthal; James A. Franz; Maciej S. Gutowski; Kenneth D. Jordan; Bruce D. Kay; Jay A. LaVerne; Sergei V. Lymar; Theodore E. Madey; C. William McCurdy; Dan Meisel; Shaul Mukamel; Anders R. Nilsson; Thomas M. Orlando; Nikolay G. Petrik; Simon M. Pimblott; James R. Rustad; Gregory K. Schenter; Sherwin J. Singer; Andrei Tokmakoff; Lai Sheng Wang; Curt Wittig; Timothy S. Zwier

doi:10.1021/cr030453x

Role of water in electron-initiated processes and radical chemistry: Issues and scientific advances

Bruce C. Garrett
, David A. Dixon
, Donald M. Camaioni
, Daniel M. Chipman
, Mark A. Johnson
, Charles D. Jonah
, Gregory A. Kimmel
, John H. Miller
, Thomas N. Rescigno
, Peter J. Rossky
, Sotiris S. Xantheas
, Steven D. Colson
, Allan H. Laufer
, Douglas Ray
, Paul F. Barbara
, David M. Bartels
, Kurt H. Becker
, Kit H. Bowen
, Stephen E. Bradforth
, Ian Carmichael

James V. Coe, L. Rene Corrales, James P. Cowin, Michel Dupuis, Kenneth B. Eisenthal, James A. Franz, Maciej S. Gutowski, Kenneth D. Jordan, Bruce D. Kay, Jay A. LaVerne, Sergei V. Lymar, Theodore E. Madey, C. William McCurdy, Dan Meisel, Shaul Mukamel, Anders R. Nilsson, Thomas M. Orlando, Nikolay G. Petrik, Simon M. Pimblott, James R. Rustad, Gregory K. Schenter, Sherwin J. Singer, Andrei Tokmakoff, Lai Sheng Wang, Curt Wittig, Timothy S. Zwier

Department of Chemical and Biological Engineering

University at Buffalo

Pacific Northwest National Laboratory
University of Alabama
University of Notre Dame
Yale University
Argonne National Laboratory
Washington State University Tri-Cities
Lawrence Berkeley National Laboratory
University of Texas at Austin
United States Department of Energy
Stevens Institute of Technology
Johns Hopkins University
University of Southern California
Ohio State University
Columbia University
Brookhaven National Laboratory
Rutgers - The State University of New Jersey, New Brunswick
University of California at Irvine
Georgia Institute of Technology
MS 69
University of California at Davis
Massachusetts Institute of Technology
Purdue University

Research output: Contribution to journal › Review article › peer-review

603 Scopus citations

Abstract

An understanding of electron-initiated processes in aqueous systems and the subsequent radical chemistry these processes induce is critical in diverse fields such as waste remediation and environmental cleanup, radiation processing, nuclear reactors, and medical diagnosis and therapy. This review outlines the opportunity in the scientific community to create a research thrust aimed at developing a fundamental understanding of electron-driven processes in aqueous systems. Successful research programs in radiation chemistry and condensed-phase chemical physics provide the foundation to build such an effort.

Original language	English
Pages (from-to)	355-389
Number of pages	35
Journal	Chemical Reviews
Volume	105
Issue number	1
DOIs	https://doi.org/10.1021/cr030453x
State	Published - Jan 2005

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10.1021/cr030453x

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Garrett, B. C., Dixon, D. A., Camaioni, D. M., Chipman, D. M., Johnson, M. A., Jonah, C. D., Kimmel, G. A., Miller, J. H., Rescigno, T. N., Rossky, P. J., Xantheas, S. S., Colson, S. D., Laufer, A. H., Ray, D., Barbara, P. F., Bartels, D. M., Becker, K. H., Bowen, K. H., Bradforth, S. E., ... Zwier, T. S. (2005). Role of water in electron-initiated processes and radical chemistry: Issues and scientific advances. Chemical Reviews, 105(1), 355-389. https://doi.org/10.1021/cr030453x

@article{bc2cee72b7e348c0a6af78a94ada9346,

title = "Role of water in electron-initiated processes and radical chemistry: Issues and scientific advances",

abstract = "An understanding of electron-initiated processes in aqueous systems and the subsequent radical chemistry these processes induce is critical in diverse fields such as waste remediation and environmental cleanup, radiation processing, nuclear reactors, and medical diagnosis and therapy. This review outlines the opportunity in the scientific community to create a research thrust aimed at developing a fundamental understanding of electron-driven processes in aqueous systems. Successful research programs in radiation chemistry and condensed-phase chemical physics provide the foundation to build such an effort.",

author = "Garrett, \{Bruce C.\} and Dixon, \{David A.\} and Camaioni, \{Donald M.\} and Chipman, \{Daniel M.\} and Johnson, \{Mark A.\} and Jonah, \{Charles D.\} and Kimmel, \{Gregory A.\} and Miller, \{John H.\} and Rescigno, \{Thomas N.\} and Rossky, \{Peter J.\} and Xantheas, \{Sotiris S.\} and Colson, \{Steven D.\} and Laufer, \{Allan H.\} and Douglas Ray and Barbara, \{Paul F.\} and Bartels, \{David M.\} and Becker, \{Kurt H.\} and Bowen, \{Kit H.\} and Bradforth, \{Stephen E.\} and Ian Carmichael and Coe, \{James V.\} and Corrales, \{L. Rene\} and Cowin, \{James P.\} and Michel Dupuis and Eisenthal, \{Kenneth B.\} and Franz, \{James A.\} and Gutowski, \{Maciej S.\} and Jordan, \{Kenneth D.\} and Kay, \{Bruce D.\} and LaVerne, \{Jay A.\} and Lymar, \{Sergei V.\} and Madey, \{Theodore E.\} and McCurdy, \{C. William\} and Dan Meisel and Shaul Mukamel and Nilsson, \{Anders R.\} and Orlando, \{Thomas M.\} and Petrik, \{Nikolay G.\} and Pimblott, \{Simon M.\} and Rustad, \{James R.\} and Schenter, \{Gregory K.\} and Singer, \{Sherwin J.\} and Andrei Tokmakoff and Wang, \{Lai Sheng\} and Curt Wittig and Zwier, \{Timothy S.\}",

year = "2005",

month = jan,

doi = "10.1021/cr030453x",

language = "English",

volume = "105",

pages = "355--389",

journal = "Chemical Reviews",

issn = "0009-2665",

publisher = "American Chemical Society",

number = "1",

}

Garrett, BC, Dixon, DA, Camaioni, DM, Chipman, DM, Johnson, MA, Jonah, CD, Kimmel, GA, Miller, JH, Rescigno, TN, Rossky, PJ, Xantheas, SS, Colson, SD, Laufer, AH, Ray, D, Barbara, PF, Bartels, DM, Becker, KH, Bowen, KH, Bradforth, SE, Carmichael, I, Coe, JV, Corrales, LR, Cowin, JP, Dupuis, M, Eisenthal, KB, Franz, JA, Gutowski, MS, Jordan, KD, Kay, BD, LaVerne, JA, Lymar, SV, Madey, TE, McCurdy, CW, Meisel, D, Mukamel, S, Nilsson, AR, Orlando, TM, Petrik, NG, Pimblott, SM, Rustad, JR, Schenter, GK, Singer, SJ, Tokmakoff, A, Wang, LS, Wittig, C & Zwier, TS 2005, 'Role of water in electron-initiated processes and radical chemistry: Issues and scientific advances', Chemical Reviews, vol. 105, no. 1, pp. 355-389. https://doi.org/10.1021/cr030453x

TY - JOUR

T1 - Role of water in electron-initiated processes and radical chemistry

T2 - Issues and scientific advances

AU - Garrett, Bruce C.

AU - Dixon, David A.

AU - Camaioni, Donald M.

AU - Chipman, Daniel M.

AU - Johnson, Mark A.

AU - Jonah, Charles D.

AU - Kimmel, Gregory A.

AU - Miller, John H.

AU - Rescigno, Thomas N.

AU - Rossky, Peter J.

AU - Xantheas, Sotiris S.

AU - Colson, Steven D.

AU - Laufer, Allan H.

AU - Ray, Douglas

AU - Barbara, Paul F.

AU - Bartels, David M.

AU - Becker, Kurt H.

AU - Bowen, Kit H.

AU - Bradforth, Stephen E.

AU - Carmichael, Ian

AU - Coe, James V.

AU - Corrales, L. Rene

AU - Cowin, James P.

AU - Dupuis, Michel

AU - Eisenthal, Kenneth B.

AU - Franz, James A.

AU - Gutowski, Maciej S.

AU - Jordan, Kenneth D.

AU - Kay, Bruce D.

AU - LaVerne, Jay A.

AU - Lymar, Sergei V.

AU - Madey, Theodore E.

AU - McCurdy, C. William

AU - Meisel, Dan

AU - Mukamel, Shaul

AU - Nilsson, Anders R.

AU - Orlando, Thomas M.

AU - Petrik, Nikolay G.

AU - Pimblott, Simon M.

AU - Rustad, James R.

AU - Schenter, Gregory K.

AU - Singer, Sherwin J.

AU - Tokmakoff, Andrei

AU - Wang, Lai Sheng

AU - Wittig, Curt

AU - Zwier, Timothy S.

PY - 2005/1

Y1 - 2005/1

N2 - An understanding of electron-initiated processes in aqueous systems and the subsequent radical chemistry these processes induce is critical in diverse fields such as waste remediation and environmental cleanup, radiation processing, nuclear reactors, and medical diagnosis and therapy. This review outlines the opportunity in the scientific community to create a research thrust aimed at developing a fundamental understanding of electron-driven processes in aqueous systems. Successful research programs in radiation chemistry and condensed-phase chemical physics provide the foundation to build such an effort.

AB - An understanding of electron-initiated processes in aqueous systems and the subsequent radical chemistry these processes induce is critical in diverse fields such as waste remediation and environmental cleanup, radiation processing, nuclear reactors, and medical diagnosis and therapy. This review outlines the opportunity in the scientific community to create a research thrust aimed at developing a fundamental understanding of electron-driven processes in aqueous systems. Successful research programs in radiation chemistry and condensed-phase chemical physics provide the foundation to build such an effort.

UR - https://www.scopus.com/pages/publications/19944430597

U2 - 10.1021/cr030453x

DO - 10.1021/cr030453x

M3 - Review article

C2 - 15720157

SN - 0009-2665

VL - 105

SP - 355

EP - 389

JO - Chemical Reviews

JF - Chemical Reviews

IS - 1

ER -

Role of water in electron-initiated processes and radical chemistry: Issues and scientific advances

Abstract

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